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Facile Synthesis of MoS2/g-C3N4/GO Ternary Heterojunction with Enhanced Photocatalytic Activity for Water Splitting
Department清洁能源化学与材料实验室
Wang M(王敏)1,2; Ju P(鞠鹏)1; Li JJ(李佳佳)1,2; Zhao Y(赵雲)1,2; Han XX(韩修训)1,3; Hao, Zhaomin4; Han XX(韩修训)
The second department青岛研发中心/青岛市资源化学与新材料研究中心
2017
Source PublicationACS Sustainable Chemistry & Engineering
ISSN2168-0485
Volume5Issue:9Pages:7878-7886
Abstract

On the basis of a simple ion exchange method, a MoS2/g-C3N4/graphene oxide (GO) ternary nanojunction was constructed as an efficient photocatalyst for hydrogen evolution using solar energy. The confinement effect in MoS2 and g-C3N4 quantum dots enhances their water-splitting redox activities. The designed heterostructure featured a band alignment that facilitates the collection of electrons in MoS2 and holes in g-C3N4, effectively suppressing the recombination of photogenerated charge carriers. Furthermore, the GO with high specific surface area serves as an excellent conductive substrate to transport holes speedily. This study thus provides a novel and facile route of establishing efficient composite photocatalyst with multinary components for energy conversion.

KeywordMos2 C3n4 Go Heterojunction Water Splitting
Subject Area材料科学与物理化学
DOI10.1021/acssuschemeng.7b01386
Funding Organizationthe National Natural Science Foundation of China (Grant 61376066;21401203);CAS “Light of West China” Program
Indexed BySCI
If5.951
Language英语
Funding Project光电材料与器件研究组
compositor第一作者单位
Citation statistics
Cited Times:132[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.licp.cn/handle/362003/22485
Collection清洁能源化学与材料实验室
青岛研发中心/青岛市资源化学与新材料研究中心
Corresponding AuthorHan XX(韩修训)
Affiliation1.Chinese Acad Sci, Lanzhou Inst Chem Phys, Lab Clean Energy Chem & Mat, 18 Tianshui Middle Rd, Lanzhou 730000, Gansu, Peoples R China
2.Univ Chinese Acad Sci, 19 Jia Yuquan Rd, Beijing 100039, Peoples R China
3.Qingdao Ctr Resource Chem & New Mat, 36 Jinshui Rd, Qingdao 266100, Peoples R China
4.Henan Univ, 85 Minglun Rd, Kaifeng 410200, Peoples R China
Recommended Citation
GB/T 7714
Wang M,Ju P,Li JJ,et al. Facile Synthesis of MoS2/g-C3N4/GO Ternary Heterojunction with Enhanced Photocatalytic Activity for Water Splitting[J]. ACS Sustainable Chemistry & Engineering,2017,5(9):7878-7886.
APA Wang M.,Ju P.,Li JJ.,Zhao Y.,Han XX.,...&韩修训.(2017).Facile Synthesis of MoS2/g-C3N4/GO Ternary Heterojunction with Enhanced Photocatalytic Activity for Water Splitting.ACS Sustainable Chemistry & Engineering,5(9),7878-7886.
MLA Wang M,et al."Facile Synthesis of MoS2/g-C3N4/GO Ternary Heterojunction with Enhanced Photocatalytic Activity for Water Splitting".ACS Sustainable Chemistry & Engineering 5.9(2017):7878-7886.
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