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Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness
Department固体润滑国家重点实验室
Ou JF(欧军飞)1; Wang, Ying3; Li, Changquan1; Wang, Fajun1; Xue MS(薛明山)1; Wang JQ(王金清)2
2013
Source PublicationSurface and Interface Analysis
ISSN0142-2421
Volume45Issue:7Pages:1182-1187
AbstractPolydopamine (coded as PDA) is reported to be very adhesive and reactive due to the attached functional groups, such as amine and hydroxyl groups. In this work, taking advantage of the condensation between Si-OH of the hydroxylated alkyltrichlorosilane (ATS) and C-OH on PDA surface, ATS molecules with different chain carbon number of 10, 14 and 18 were grafted onto the 3-aminopropyl triethoxysilane (APTES)-PDA dual-layer film, which was composed of PDA outerlayer and APTES underlayer, on Si substrate. Thus, hydrophobic trilayer films coded as APTES-PDA-ATS were prepared successfully. In order to reveal the dependence of the tribological behaviors upon the microstructures of the film, tribological experiments were conducted on an atomic force microscope and a ball-on-plate tribometer. Experimental results showed that the (micro-) friction reducing (characterized by a parameter of relative friction coefficient or friction coefficient, RFC or FC) and macro-wear resisting (characterized by anti-wear life) behaviors were related with the chain length of outerlayer and the PDA thickness. Specifically, on one hand, as the chain length increases, RFC/FC decreased and macro anti-wear life lengthened; on the other hand, as PDA gets thicker, RFC increased and the anti-wear life enhanced.
KeywordPolydopamine Tribological Performances Surface Grafting
Subject Area材料科学与物理化学
DOI10.1002/sia.5246
Funding Organizationthe National Natural Science Foundation of China (Grant No. 21203089);Jiangxi provincial department of science and technology (Grant No. 20123BDH80015)
Indexed BySCI
If1.393
Language英语
Funding Project聚合物摩擦学组
compositor第二作者单位
Citation statistics
Cited Times:3[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.licp.cn/handle/362003/18179
Collection固体润滑国家重点实验室(LSL)
Affiliation1.Nanchang Hangkong Univ, Sch Mat Sci & Engn, Nanchang 330063, Peoples R China
2.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China
3.Jiangsu Key Lab Solar Cell Mat & Technol, Changzhou 213164, Peoples R China
Recommended Citation
GB/T 7714
Ou JF,Wang, Ying,Li, Changquan,et al. Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness[J]. Surface and Interface Analysis,2013,45(7):1182-1187.
APA Ou JF,Wang, Ying,Li, Changquan,Wang, Fajun,Xue MS,&Wang JQ.(2013).Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness.Surface and Interface Analysis,45(7),1182-1187.
MLA Ou JF,et al."Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness".Surface and Interface Analysis 45.7(2013):1182-1187.
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