Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness | |
Department | 固体润滑国家重点实验室 |
Ou JF(欧军飞)1; Wang, Ying3; Li, Changquan1; Wang, Fajun1; Xue MS(薛明山)1; Wang JQ(王金清)2 | |
2013 | |
Source Publication | Surface and Interface Analysis |
ISSN | 0142-2421 |
Volume | 45Issue:7Pages:1182-1187 |
Abstract | Polydopamine (coded as PDA) is reported to be very adhesive and reactive due to the attached functional groups, such as amine and hydroxyl groups. In this work, taking advantage of the condensation between Si-OH of the hydroxylated alkyltrichlorosilane (ATS) and C-OH on PDA surface, ATS molecules with different chain carbon number of 10, 14 and 18 were grafted onto the 3-aminopropyl triethoxysilane (APTES)-PDA dual-layer film, which was composed of PDA outerlayer and APTES underlayer, on Si substrate. Thus, hydrophobic trilayer films coded as APTES-PDA-ATS were prepared successfully. In order to reveal the dependence of the tribological behaviors upon the microstructures of the film, tribological experiments were conducted on an atomic force microscope and a ball-on-plate tribometer. Experimental results showed that the (micro-) friction reducing (characterized by a parameter of relative friction coefficient or friction coefficient, RFC or FC) and macro-wear resisting (characterized by anti-wear life) behaviors were related with the chain length of outerlayer and the PDA thickness. Specifically, on one hand, as the chain length increases, RFC/FC decreased and macro anti-wear life lengthened; on the other hand, as PDA gets thicker, RFC increased and the anti-wear life enhanced. |
Keyword | Polydopamine Tribological Performances Surface Grafting |
Subject Area | 材料科学与物理化学 |
DOI | 10.1002/sia.5246 |
Funding Organization | the National Natural Science Foundation of China (Grant No. 21203089);Jiangxi provincial department of science and technology (Grant No. 20123BDH80015) |
Indexed By | SCI |
If | 1.393 |
Language | 英语 |
Funding Project | 聚合物摩擦学组 |
compositor | 第二作者单位 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.licp.cn/handle/362003/18179 |
Collection | 固体润滑国家重点实验室(LSL) |
Affiliation | 1.Nanchang Hangkong Univ, Sch Mat Sci & Engn, Nanchang 330063, Peoples R China 2.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China 3.Jiangsu Key Lab Solar Cell Mat & Technol, Changzhou 213164, Peoples R China |
Recommended Citation GB/T 7714 | Ou JF,Wang, Ying,Li, Changquan,et al. Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness[J]. Surface and Interface Analysis,2013,45(7):1182-1187. |
APA | Ou JF,Wang, Ying,Li, Changquan,Wang, Fajun,Xue MS,&Wang JQ.(2013).Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness.Surface and Interface Analysis,45(7),1182-1187. |
MLA | Ou JF,et al."Tribological behaviors of a novel trilayer nanofilm: the influence of outer chain length and interlayer thickness".Surface and Interface Analysis 45.7(2013):1182-1187. |
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LZ01027651.pdf(434KB) | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | View Application Full Text |
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