| Photocatalytic H2 evolution from NaCl saltwater over ZnS1-x-0.5yOx(OH)y-ZnO under visible light irradiation | |
| Department | 羰基合成与选择氧化国家重点实验室 ; 精细石油化工中间体国家工程研究中心 |
Li YX(李越湘); He F(何芳); Peng SQ(彭绍琴); Lv GX(吕功煊) ; Li SB(李树本)
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| 2011 | |
| Source Publication | Int. J. Hydrog. Energy
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| ISSN | 0360-3199 |
| Volume | 36Pages:10565-10573 |
| Abstract | Photocatalytic hydrogen production was investigated over ZnS1 x 0.5yOx(OH)yeZnO using sulfide ion (Na2SeNa2SO3) as an electron donor from NaCl saltwater. NaCl can affect markedly the activity for photocatalytic hydrogen production, depending on NaCl concentration. When NaCl concentration is lower, the activity is lower than that in pure water, whereas when NaCl concentration is higher, the activity is higher than that in pure water. NaCl decreases not only the surface charge of ZnS1 x 0.5yOx(OH)yeZnO but also the surface hydration. When ZnS1 x 0.5yOx(OH)yeZnO was impregnated with the electron donor (Na2SeNa2SO3), ZnO was transformed partly into ZnS. The impregnated ZnS1 x 0.5y Ox(OH)yeZnO exhibits higher activity than the non-impregnated one. The possible mechanisms were discussed. |
| Keyword | Zns1 x 0.5yox(Oh)Y-zno Hydrogen Evolution Sodium Chloride Sulfide Ion Impregnation |
| Subject Area | 物理化学 |
| Funding Organization | the National Basic Research Program of China (2009CB220003);the National Nature Science Foundation of China (No. 20763006);Specialized Research Fund for the Doctoral Program of Higher Education of China (20060403006);the Natural Science Foundation of the Jiangxi Province (2010JZH0096);Research Fund of Education Ministry of Jiangxi, China (GJJ09041) |
| Indexed By | SCI |
| Language | 英语 |
| Funding Project | 环境催化与氢能研究组 ; 环境催化与氢能源研究组 |
| Document Type | 期刊论文 |
| Identifier | http://ir.licp.cn/handle/362003/381 |
| Collection | 羰基合成与选择氧化国家重点实验室（OSSO） 精细石油化工中间体国家工程研究中心（ERC） |
| Corresponding Author | Li YX(李越湘) |
| Recommended Citation GB/T 7714 | Li YX,He F,Peng SQ,et al. Photocatalytic H2 evolution from NaCl saltwater over ZnS1-x-0.5yOx(OH)y-ZnO under visible light irradiation[J]. Int. J. Hydrog. Energy,2011,36:10565-10573. |
| APA | 李越湘,何芳,彭绍琴,吕功煊,&李树本.(2011).Photocatalytic H2 evolution from NaCl saltwater over ZnS1-x-0.5yOx(OH)y-ZnO under visible light irradiation.Int. J. Hydrog. Energy,36,10565-10573. |
| MLA | 李越湘,et al."Photocatalytic H2 evolution from NaCl saltwater over ZnS1-x-0.5yOx(OH)y-ZnO under visible light irradiation".Int. J. Hydrog. Energy 36(2011):10565-10573. |
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