| Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania | |
| Department | OSSO国家重点实验室 |
Song AY(宋爱英)1,2,3; Lu GX(吕功煊)1 ; Lv GX(吕功煊)
| |
| The second department | erc国家工程研究中心 |
| 2015 | |
| Source Publication | Environmental Technology
 |
| ISSN | 0959-3330 |
| Volume | 36Issue:9Pages:1160-1166 |
| Abstract | Promotion of the dispersion of Ru species supported on TiO2 was achieved by introduction of Pt component and the role of Pt in enhancing the catalytic performances of Pt–Ru was investigated with catalytic wet air oxidation of methylamine used as a probing reaction. It was found that Pt–Ru/TiO2 displayed a much better catalytic performance compared with Pt/TiO2 and Ru/TiO2 catalysts due to having the highest dispersion of active species. Both high total organic carbon conversion and nitrogen selectivity (∼100%) over Pt–Ru/TiO2 catalyst were achieved at low temperature (200 °C). X-ray photoelectron spectroscopy characterization indicated that there were strong interactions between metal particles and the support, which may increase the catalytic performance of catalysts. |
| Keyword | Methylamine Pt-ru Cwao Dispersion Tio2 |
| Subject Area | 物理化学与绿色催化 |
| DOI | 10.1080/09593330.2014.982721 |
| Funding Organization | the National Science Foundation of China (Grant Nos.21373245;21173242);973 and 863 Program of Department of Sciences and Technology of China (Grant Nos. 2013CB632404;2012AA051501;2009CB22003);Gansu Provincial Science & Technology Department (1304FKCA085) |
| Indexed By | SCI |
| If | 1.760 |
| Language | 英语 |
| Funding Project | 环境催化与氢能源研究组;环境催化与清洁能源研究组 |
| compositor | 第一作者单位 |
| Citation statistics | |
| Document Type | 期刊论文 |
| Identifier | http://ir.licp.cn/handle/362003/19304 |
| Collection | 羰基合成与选择氧化国家重点实验室（OSSO） 精细石油化工中间体国家工程研究中心（ERC） |
| Corresponding Author | Lv GX(吕功煊) |
| Affiliation | 1.Univ Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Oxo Synth & Select Oxidat, Lanzhou 730000, Peoples R China 2.Gansu Inst Polit Sci & Law, Coll Publ Secur Technol, Lanzhou 730070, Peoples R China 3.Phys Chem Lab Gansu Prov Ctr Dis Control & Preven, Lanzhou 730020, Peoples R China |
| Recommended Citation GB/T 7714 | Song AY,Lu GX,Lv GX. Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania[J]. Environmental Technology,2015,36(9):1160-1166. |
| APA | Song AY,Lu GX,&吕功煊.(2015).Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania.Environmental Technology,36(9),1160-1166. |
| MLA | Song AY,et al."Catalytic wet oxidation of aqueous methylamine: comparative study on the catalytic performance of platinum-ruthenium, platinum, and ruthenium catalysts supported on titania".Environmental Technology 36.9(2015):1160-1166. |
| Files in This Item: | ||||||
| File Name/Size | DocType | Version | Access | License | ||
| LZ01028428.pdf（6878KB） | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | View Application Full Text | |
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