pH-Responsive Controlled-Release Fertilizer with Water Retention via Atom Transfer Radical Polymerization of Acrylic Acid on Mussel-Inspired Initiator | |
Department | 固体润滑国家重点实验室 |
Ma, Zhi-yuan1; Jia, Xin1; Zhang, Guo-xiang1; Hu, Jia-mei1; Zhang, Xiu-lan1; Liu, Zhi-yong1; Wang, He-yun1; Zhou F(周峰)2 | |
2013 | |
Source Publication | Journal of Agricultural and Food Chemistry |
ISSN | 0021-8561 |
Volume | 61Issue:23Pages:5474-5482 |
Abstract | This work reports a polydopamine-graft-poly(acrylic acid) (Pdop-g-PAA)-coated controlled-release multi-element compound fertilizer with water-retention function by a combination of mussel-inspired chemistry and surface-initiated atom transfer radical polymerization (SI-ATRP) techniques for the first time The morphology and composition of the products were characterized by transmission electron microscopy (TEM), Fourier transform infrared (FTIR) spectroscopy, thermogravimetric analysis (TGA), gel permeation chromatography (GPC), and inductively coupled plasma (ICP) emission spectrometry. The results revealed that the stimuli responsive layer formed by a Pdop inner layer and a PAA outer corona exhibit outstanding selective permeability to charged nutrients and the release rate of encapsulated elements can be tailored by the pH values. At low pH, the Pdop-g-PAA layer can reduce nutrient loss, and at high pH, the coating restrains transportation of negative nutrients but favors the release of cations. Moreover, PAA brushes provide good water retention property. This Pdop-graft-polymer brushes coating will be effective and promising in the research and development of multi functional controlled release fertilizer. |
Keyword | Controlled Release Fertilizer Polydopamine Ph-responsive Poly(Acrylic Acid) Atom Transfer Radical Polymerization |
Subject Area | 材料科学与物理化学 |
DOI | 10.1021/jf401102a |
Funding Organization | the National Natural Science Foundation of China (21264013) |
Indexed By | SCI |
If | 3.107 |
Language | 英语 |
Funding Project | 材料表面与界面行为研究组 |
compositor | 第二作者单位 |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.licp.cn/handle/362003/18200 |
Collection | 固体润滑国家重点实验室(LSL) |
Affiliation | 1.Shihezi Univ, Key Lab Green Proc Chem Engn Xinjiang Bingtuan, Key Lab Chem Mat Xinjiang Uygur Autonomous Reg, Sch Chem & Chem Engn, Shihezi 832003, Peoples R China 2.Chinese Acad Sci, Lanzhou Inst Chem Phys, State Key Lab Solid Lubricat, Lanzhou 730000, Peoples R China |
Recommended Citation GB/T 7714 | Ma, Zhi-yuan,Jia, Xin,Zhang, Guo-xiang,et al. pH-Responsive Controlled-Release Fertilizer with Water Retention via Atom Transfer Radical Polymerization of Acrylic Acid on Mussel-Inspired Initiator[J]. Journal of Agricultural and Food Chemistry,2013,61(23):5474-5482. |
APA | Ma, Zhi-yuan.,Jia, Xin.,Zhang, Guo-xiang.,Hu, Jia-mei.,Zhang, Xiu-lan.,...&Zhou F.(2013).pH-Responsive Controlled-Release Fertilizer with Water Retention via Atom Transfer Radical Polymerization of Acrylic Acid on Mussel-Inspired Initiator.Journal of Agricultural and Food Chemistry,61(23),5474-5482. |
MLA | Ma, Zhi-yuan,et al."pH-Responsive Controlled-Release Fertilizer with Water Retention via Atom Transfer Radical Polymerization of Acrylic Acid on Mussel-Inspired Initiator".Journal of Agricultural and Food Chemistry 61.23(2013):5474-5482. |
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LZ01027659.pdf(518KB) | 期刊论文 | 作者接受稿 | 开放获取 | CC BY-NC-SA | View Application Full Text |
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